بررسی توانایی هیدروکسید دوگانه لایه‌ای Ni/Al سنتزشده در حذف رنگ تارترازین

نوع مقاله : مقاله پژوهشی

نویسندگان

گروه شیمی، دانشکده علوم پایه، دانشگاه آزاد اسلامی واحد خرم‌آباد، خرم‌آباد، ایران، صندوق پستی: 68135/536

چکیده

در این پژوهش نخست هیدروکسید دوگانه لایه­ای Ni/Al به روش هم­رسوبی سنتز شده و سپس به عنوان جاذب برای حذف رنگ تارترازین از محلول آبی استفاده شده است. مشخصه­یابی جاذب سنتزی توسط پراش پرتو ایکس و میکروسکوپ الکترونی روبشی انجام شد. در مطالعه فرآیند جذب سطحی بهینه­سازی غلظت اولیه رنگ، زمان تماس، pH، مقدار جاذب و دما انجام گرفت. مقدار درصد حذف رنگ در شرایط بهینه 98 درصد و بیشینه ظرفیت جذب برابر mg.g-1 3333.33 بود. بررسی­های سینتیکی جذب سطحی بیانگر همخوانی این فرآیند از سینتیک شبه مرتبه اول می­باشد. مطالعات ترمودینامیکی این پژوهش نشان داد فرآیند حذف رنگ توسط جاذب سنتزی، گرماده و خودبه­خودی بوده که همراه با کاهش بی­نظمی است. داده­های به­دست آمده گویای این است که هیدروکسید دوگانه لایه­ای Ni/Al می­تواند جاذب کارآمدی برای حذف تارترازین از محلول آبی باشد.

کلیدواژه‌ها

عنوان مقاله [English]

Investigation of the Ability of Synthesized Layered Double Hydroxide Ni/Al to Remove Tartrazine Dye

نویسندگان [English]

  • A. Ahmadi Iranshahi
  • Ghazaleh Kouchakzadeh
Department of Chemistry, Islamic Azad University, Khorramabad branch, P.O.Box: 536/68135, Khorramabad, Iran
چکیده [English]

In this research, the first layered double hydroxide Ni­/Al was synthesized by co­-precipitation method, and then it was used to remove tartrazine dye from an aqueous solution. The synthesized adsorbent was characterized by X-ray diffraction and a scanning electron microscope. Initial concentration, contact time, pH, the dose of adsorbent and temperature were optimized in this adsorption process. The dye removal percentage and maximum adsorption capacity were 98 % and 3333.33 mg.g-1, respectively. The results showed that the adsorption kinetics follow pseudo­-­first­-­order model. According to thermodynamic results, the process of dye removal by synthesized adsorbent is exothermic, spontaneous, and accompanied by decreasing irregularity. This research showed that layered double hydroxide Ni­-­Al could be an efficient adsorbent for tartrazine removal from an aqueous solution.

کلیدواژه‌ها [English]

  • Dye removal Layered double hydroxide Ni‌/Al Tartrazine dye Pseudo
  • first
  • order kinetics

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